Hello Mezzofan
Thank you for your contribution to the Microsoft Community.
I understand that you want to add a custom dictionary but Word crashes. This must have caused problems in your life and work.
First, I need to confirm some information:
The version of Word you are using. File>Account. Please provide a screenshot if it is convenient.
You mentioned that Word crashed. Is there an error message? Is there a record in the Event Viewer? Please provide a screenshot if it is convenient.
Does this problem only occur in this one file? or does it occur in all Word files? Please create a new file to test.
Here's a tutorial for adding a custom dictionary:
Add or edit words in a spell check dictionary - Microsoft Support
You have tried to fix or even reinstall Microsoft 365. I will give some other scenarios:
Cancel the add-on
Click the file > option in the upper left corner of the document> change the place where Add-ons > Management to COM Add-ins> then select "Go", uncheck all add-ins > click OK > restart the word document and see the effect.
Delete the Word template
Close all documents, press Windows + R, type %AppData%MicrosoftTemplates in the run box that opens, press enter,
Back up and delete files with .dotm suffix, such as Normal.dotm, and then reopen the word document attempt
Registry reset Office
Press Windows + R, type regedit in the run box that opens, press enter,
Rename the Office folder by navigating to the following key (right-click on it and select Rename, e.g. Rename Office to Officeold)
HKEY_CURRENT_USER\Software\Microsoft\Office
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Then reopen the word document to try the effect.
Disclaimer: Generally, modifying registry subkeys or work group is intended for advanced users, administrators, and IT Professionals. It can help fix some problems, however, serious problems might occur if you modify the registry incorrectly. Therefore, make sure that you follow these steps carefully. For further protection, back up the registry before you modify it. Then, you can restore the registry if a problem occurs. For more information about how to back up and restore the registry, click here to view the article.
How to back up and restore the registry in Windows - Microsoft Support
If there is a mistake in my understanding, please describe it in more detail. Looking forward to your further reply so that we can serve you better.
Best wishes,
Rel - MSFT | Microsoft Community Support Specialist